A Large-Eddy Simulation Study of Water Vapour and Carbon Dioxide Isotopes in the Atmospheric Boundary Layer
A large-eddy simulation model developed at the National Center for Atmospheric Research (NCAR) is extended to simulate the transport and diffusion of C¹â¸OO, Hâ¹â¸O and ¹³COâ in the atmospheric boundary layer (ABL). The simulation results show that the ¹â¸O compositions of leaf water and the ABL COâ are moderately sensitive to wind speed. The variations in the ¹â¸O composition of water vapour are an order of magnitude greater than those in the ¹³C and ¹â¸O compositions of COâ both at turbulent eddy scales and across the capping inversion. In a fully-developed convective ABL, these isotopic compositions are well mixed as with other conserved atmospheric quantities. The Keeling intercepts determined with the simulated high-frequency turbulence time series do not give a reliable estimate of the ¹â¸O composition of the surface water vapour flux and may be a reasonable approximation to the ¹³C and ¹â¸O compositions of the surface COâ flux in the late afternoon only after a deep convective ABL has developed. We suggest that our isotopic large-eddy simulation (ISOLES) model should be a useful tool for testing and formulating research hypotheses on landâair isotopic exchanges.
document
https://n2t.org/ark:/85065/d7hh6kt1
eng
geoscientificInformation
Text
publication
2016-01-01T00:00:00Z
publication
2012-10-01T00:00:00Z
Copyright 2012 Springer.
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