Evaluating ethane and methane emissions associated with the development of oil and natural gas extraction in North America
Sharp rises in the atmospheric abundance of ethane (CâHâ) have been detected from 2009 onwards in the Northern Hemisphere as a result of the unprecedented growth in the exploitation of shale gas and tight oil reservoirs in North America. Using time series of CâHâ total columns derived from ground-based Fourier transform infrared (FTIR) observations made at five selected Network for the Detection of Atmospheric Composition Change sites, we characterize the recent CâHâ evolution and determine growth rates of ~5% yrâ»Â¹ at mid-latitudes and of ~3% yrâ»Â¹ at remote sites. Results from CAM-chem simulations with the Hemispheric Transport of Air Pollutants, Phase II bottom-up inventory for anthropogenic emissions are found to greatly underestimate the current CâHâ abundances. Doubling global emissions is required to reconcile the simulations and the observations prior to 2009. We further estimate that North American anthropogenic CâHâ emissions have increased from 1.6 Tg yrâ»Â¹ in 2008 to 2.8 Tg yrâ»Â¹ in 2014, i.e. by 75% over these six years. We also completed a second simulation with new top-down emissions of CâHâ from North American oil and gas activities, biofuel consumption and biomass burning, inferred from space-borne observations of methane (CHâ) from Greenhouse Gases Observing SATellite. In this simulation, GEOS-Chem is able to reproduce FTIR measurements at the mid-latitudinal sites, underscoring the impact of the North American oil and gas development on the current CâHâ abundance. Finally we estimate that the North American oil and gas emissions of CHâ, a major greenhouse gas, grew from 20 to 35 Tg yrâ»Â¹ over the period 2008-2014, in association with the recent CâHâ rise.
document
https://n2t.org/ark:/85065/d7dz09vf
eng
geoscientificInformation
Text
publication
2016-01-01T00:00:00Z
publication
2016-04-07T00:00:00Z
Copyright 2016 IOP Publishing Ltd.
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